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Department of Decommissioning and Waste Management
JAEA-Review 2023-001, 136 Pages, 2023/06
This report describes the activities of Department of Decommissioning and Waste Management (DDWM) in Nuclear Science Research Institute (NSRI) in the period from April 1, 2021 to March 31, 2022. The report covers organization and missions of DDWM, outline and operation/maintenance of facilities which belong to DDWM, treatment and management of radioactive wastes, decommissioning activities, and related research and development activities which were conducted in DDWM. In FY2021 radioactive wastes generated from R&D activities in NSRI were treated safely. They were about 206 m of combustible solid wastes and 155 m of noncombustible solid wastes and 113 m of liquid wastes. After adequate treatment, 760 waste packages (in 200 L-drum equivalent) were generated. The total amounts of accumulated waste packages were 126,827 as of the end of FY2021 due to efforts of the restitution of waste packages to the Japan Radioisotope Association and volume reduction treatments of the stored waste packages. Decommissioning activities were carried out for the JAEA's Reprocessing Test Facility (JRTF), the Liquid Waste Treatment Facilities, the Compaction Facilities, and Fusion Neutronics Source (FNS) facilities. As for the R&D activities, studies on radiochemical analyses of wastes for disposal were continued. In order to pass the conformity review on the New Regulatory Requirements for waste management facilities, the Approval of the design and construction method was applied sequentially for the Nuclear Regulation Authority. The ministry of the Environment and Tokai-mura office requested JAEA to dispose of the contaminated soil generated by the accident of the Fukushima Daiichi Nuclear Power Station. The monitoring work at the playground was conducted during this period.
Collaborative Laboratories for Advanced Decommissioning Science; Shibaura Institute of Technology*
JAEA-Review 2022-008, 116 Pages, 2022/06
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2018, this report summarizes the research results of the "Development of the sintering solidification method for spent zeolite to long-term stabilization" conducted from FY2018 to FY2021 (this contract was extended to FY2021). Since the final year of this proposal was FY2021, the results for four fiscal years were summarized. The present study aims to develop a new sintering solidification method in which glass is added as a binder to spent zeolite which is adsorbed radionuclides such as Cs and the nuclides are immobilized by sintering them. In this project, the optimum conditions for sintering solidification and the basic performance of the sintered solidified body will be evaluated by cold tests, and they will be demonstrated by hot tests.
Ochs, M.*; Dolder, F.*; Tachi, Yukio
Applied Geochemistry, 136, p.105161_1 - 105161_11, 2022/01
Times Cited Count:4 Percentile:63.38(Geochemistry & Geophysics)Various types of radioactive wastes and environments contain organic substances that can stabilize the aqueous complexes with radionuclides and therefore lead to a decrease of sorption. The present study focuses on testing a methodology to quantify sorption reduction factors (SRFs) in the presence of organic ligands for cement systems. Three approaches for the estimation of SRFs; (1) analogy with solubility enhancement factors, (2) radionuclide speciation based on the thermodynamic calculations, and (3) experimental sorption data in ternary systems, were coupled and tested for the representative organic ligands (ISA and EDTA) and selected key radionuclides (actinides). Our approach allows to critically evaluate the dependence of SRFs for various systems on the chosen method of quantification, in accordance with the data availability for a given systems. The reliable SRFs can only be derived from the sorption measurements in ternary systems. SRF often need to be derived in the absence of such direct evidence, and estimations need to be made based on analogies and speciation information. However, such estimates may be subject to substantial uncertainties.
Collaborative Laboratories for Advanced Decommissioning Science; University of Tsukuba*
JAEA-Review 2021-023, 49 Pages, 2021/12
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2018, this report summarizes the research results of the "Upgrading of recovery method for radioactive microparticles by heavy liquid separation aiming to volume reduction of contaminated soil" conducted from FY2018 to FY2020. Since the final year of this proposal was FY2020, the results for three fiscal years were summarized. The present study aims to develop a novel method to reduce the volume of contaminated soil caused by an accident at the Fukushima Daiichi Nuclear Power Station. The heavy liquid separation method, which was optimized in the previous year, was applied to nine soils collected in Fukushima Prefecture.
Kato, Takuma*; Nagaoka, Mika; Guo, H.*; Fujita, Hiroki; Aida, Taku*; Smith, R. L. Jr.*
Environmental Science and Pollution Research, 28(39), p.55725 - 55735, 2021/10
Times Cited Count:0 Percentile:0(Environmental Sciences)In this work, hydrothermal leaching was applied to simulated soils (clay minerals vermiculite, montmorillonite, kaolinite) and actual soils (Terunuma, Japan) to generate organic acids with the objective to develop an additive-free screening method for determination of Sr in soil. Stable strontium (SrCl) was adsorbed onto soils for study and ten organic acids were evaluated for leaching Sr from simulated soils under hydrothermal conditions (120 to 200C) at concentrations up to 0.3 M. For strontium-adsorbed vermiculite (Sr-V), 0.1 M citric acid was found to be effective for leaching Sr at 150C and 1 h treatment time. Based on these results, the formation of organic acids from organic matter in Terunuma soil was studied. Hydrothermal treatment of Terunuma soil produced a maximum amount of organic acids at 200C and 0.5 h reaction time. To confirm the possibility for leaching of Sr from Terunuma soil, strontium-adsorbed Terunuma soil (Sr-S) was studied. For Sr-S, hydrothermal treatment at 200C for 0.5 h reaction time allowed 40% of the Sr to be leached at room temperature, thus demonstrating an additive-free method for screening of Sr in soil. The additive-free hydrothermal leaching method avoids calcination of solids in the first step of chemical analysis and has application to both routine monitoring of metals in soils and to emergency situations.
Collaborative Laboratories for Advanced Decommissioning Science; Shibaura Institute of Technology*
JAEA-Review 2020-049, 78 Pages, 2021/01
JAEA/CLADS had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project. Among the adopted proposals in FY2018, this report summarizes the research results of the "Development of the Sintering Solidification Method for Spent Zeolite to Long-term Stabilization" conducted in FY2019.
Department of Decommissioning and Waste Management
JAEA-Review 2020-012, 103 Pages, 2020/08
This report describes the activities of Department of Decommissioning and Waste Management (DDWM) in Nuclear Science Research Institute (NSRI) in the period from April 1, 2018 to March 31, 2019. The report covers organization and missions of DDWM, outline and operation/maintenance of facilities which belong to DDWM, treatment and management of radioactive wastes, decommissioning activities, and related research and development activities which were conducted in DDWM.
Collaborative Laboratories for Advanced Decommissioning Science; Shibaura Institute of Technology*
JAEA-Review 2019-028, 71 Pages, 2020/03
JAEA/CLADS, had been conducting the Center of World Intelligence Project for Nuclear Science/Technology and Human Resource Development (hereafter referred to "the Project") in FY2018. Among the adopted proposals in FY2018, this report summarizes the research results of the "Development of the Sintering Solidification Method for Spent Zeolite to Long-term Stabilization". The present study aims to develop the sintering solidification method for zeolites (spent zeolites) that adsorbs continuously generated radionuclides such as cesium. The sintering solidification method is able to stabilize adsorbed radionuclides such as cesium in zeolites by adding a glass as a binder to spent zeolite and sintered it. It is expected that the sintering solidification method is significantly reduce the volume of the solidified body compare with the glass solidification method and to form a stable solidified body equivalent to the calcination solidification method. In this project, we planned to select a glass suitable for the sintering solidification method and optimize the sintering temperature, etc. using non-radioactive nuclides (cold tests), and verify it by using radioactive nuclides (hot tests). In FY2018, we investigated the thermal properties of candidate glasses for binder and the effect of heating atmosphere on the sintering solidification method. Irradiated fuel for preparing simulated contaminated water containing radionuclides was selected and the condition of it was observed. In addition, we surveyed existing research results and latest research trends about solidification of zeolite, calcination solidification and so on.
Department of Decommissioning and Waste Management
JAEA-Review 2019-011, 91 Pages, 2019/10
This report describes the activities of Department of Decommissioning and Waste Management (DDWM) in Nuclear Science Research Institute (NSRI) in the period from April 1, 2017 to March 31, 2018. The report covers organization and missions of DDWM, outline and operation/maintenance of facilities which belong to DDWM, treatment and management of radioactive wastes, decommissioning activities, and related research and development activities which were conducted in DDWM.
Tachi, Yukio; Ochs, M.*
Progress in Nuclear Science and Technology (Internet), 5, p.229 - 232, 2018/11
Various types of post-accident radioactive waste have been generated from cleanup and decommissioning activities at the Fukushima Daiichi Nuclear Power Plant. For the disposal of these wastes, perturbation effects resulting from co-existing substances (e.g., organic substances, boron, and salts) are needed to be considered. Such co-existing substances may influence on the radionuclide sorption parameters for the safety assessment of the disposal systems. The present study focuses on developing the methodology to quantify sorption parameters by considering such perturbation effects and illustrating example calculations regarding the sorption reduction factors (SRFs) due to the presence of organic ligands (ISA) for cement systems. Three approaches for the derivations of SRFs for cement-Am-ISA case were compared. These options should be applied as a stepwise manner according to the data availability for the perturbation effects resulting from the co-existing substances.
Department of Decommissioning and Waste Management
JAEA-Review 2018-008, 87 Pages, 2018/07
This report describes the activities of Department of Decommissioning and Waste Management (DDWM) in Nuclear Science Research Institute (NSRI) in the period from April 1, 2016 to March 31, 2017. The report covers organization and missions of DDWM, outline and operation/maintenance of facilities which belong to DDWM, treatment and management of radioactive wastes, decommissioning activities, and related research and development activities which were conducted in DDWM.
Department of Decommissioning and Waste Management
JAEA-Review 2016-029, 90 Pages, 2017/02
This report describes the activities of Department of Decommissioning and Waste Management (DDWM) in Nuclear Science Research Institute (NSRI) in the period from April 1, 2015 to March 31, 2016. The report covers organization and missions of DDWM, outline and operation/maintenance of facilities which belong to DDWM, treatment and management of radioactive wastes, decommissioning activities, and related research and development activities which were conducted in DDWM.
Department of Decommissioning and Waste Management
JAEA-Review 2015-004, 90 Pages, 2015/03
This report describes the activities of Department of Decommissioning and Waste Management (DDWM) in Nuclear Science Research Institute (NSRI) in the period from April 1, 2013 to March 31, 2014. The report covers organization and missions of DDWM, outline and operation/maintenance of facilities which belong to DDWM, treatment and management of radioactive wastes, decommissioning activities, and related research and development activities which were conducted in DDWM.
Irisawa, Keita; Komatsuzaki, Toshio; Kawato, Yoshimi; Sakakibara, Tetsuro; Nakazawa, Osamu; Meguro, Yoshihiro
JAEA-Technology 2014-039, 28 Pages, 2014/12
In JAEA, 13,296 drums of low-radioactivity bituminized waste products (BWPs) have been stored in asphalt solidification storages. In order to effectively utilize the space of the BWP in a repository site, we studied refilling techniques of the BWP from the drum to a box-shaped container. Tentative processes, which we devised, consisted of (1) take-off of BWP from the drum, (2) separation of a post filling part from BWP and (3) filling of BWP to a box-shaped container. Two methods for each process were selected, and work efficiencies of the methods were investigated by using a synthetic BWP.
Higuchi, Hidekazu; Momma, Toshiyuki; Nakashio, Nobuyuki; Kozawa, Kazushige; Tohei, Toshio; Sudo, Tomoyuki; Mitsuda, Motoyuki; Kurosawa, Shigenobu; Hemmi, Ko; Ishikawa, Joji; et al.
Proceedings of International Conference on Nuclear Energy System for Future Generation and Global Sustainability (GLOBAL 2005) (CD-ROM), 6 Pages, 2005/10
The JAERI constructed the Advanced Volume Reduction Facilities(AVRF). The AVRF consists of the Waste Size Reduction and Storage Facilities(WSRSF) and the Waste Volume Reduction Facilities(WVRF). By operating the AVRF, it will be able to produce waste packages for final disposal and to reduce the amount of the low level solid wastes. Cutting installations for large wastes such as tanks in the WSRSF have been operating since June 1999. The wastes treated so far amount to 600 m and the volume reduction ratio is around 1/3. The waste volume reduction is carried out by a high-compaction process or melting processes in the WVRF. The metal wastes from research reactors are treated by the high-compaction process. The other wastes are treated by the melting processes that enable to estimate radioactivity levels easily by homogenization and get chemical and physical stability. The WVRF have been operating with non-radioactive wastes since February 2003 for the training and the homogeneity investigation in the melting processes. The operation with radioactive wastes will start in FY2005.
Uchiyama, Gunzo; Maeda, Mitsuru; Fujine, Sachio; *; *; *
Journal of Nuclear Science and Technology, 31(3), p.228 - 239, 1994/03
Times Cited Count:8 Percentile:60.14(Nuclear Science & Technology)no abstracts in English
; *; *; *; *; *; Kimura, Hideo; Munakata, Masahiro
Nihon Genshiryoku Gakkai-Shi, 34(4), p.342 - 364, 1992/04
Times Cited Count:2 Percentile:27.46(Nuclear Science & Technology)no abstracts in English
Uchiyama, Gunzo; *; ; *; Sugikawa, Susumu; Maeda, Mitsuru; Tsujino, Takeshi
Radioact. Waste Manage. Nucl. Fuel Cycle, 17(1), p.63 - 79, 1992/00
no abstracts in English
Uchiyama, Gunzo; *; ; Sugikawa, Susumu; Maeda, Mitsuru; Tsujino, Takeshi
JAERI-M 91-199, 35 Pages, 1991/11
no abstracts in English
Ishigami, Tsutomu; Homma, Toshimitsu
JAERI-M 89-111, 27 Pages, 1989/09
no abstracts in English